The material is arranged into six series, some of which are further divided into subseries. More detailed information on each level of organization is provided by the scope and content notes for the collection as a whole and for the individual series and subseries.
Series I. Correspondence, 1958-2009
Series II. Lectures, 1981-2007
Series III. Shimony Manuscripts, 1950-2007
Series IV. Manuscripts Annotated by Shimony, undated
Series V. National Science Foundation, undated
Series VI. Library, 1958-2007